Liquid exfoliated SnP3 nanosheets for very high areal capacity Lithium-Ion Batteries
Increasing the energy density of lithium-ion batteries requires the discovery of new electrode materials capable of achieving very high areal capacity. Here, liquid phase exfoliation is used to produce nanosheets of SnP3, a 2D material with extremely high theoretical capacity of 1670 mAh g−1. These...
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| Main Authors: | , , , , , , , , , , , , , , , , |
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| Format: | Article (Journal) |
| Language: | English |
| Published: |
2021
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| In: |
Advanced energy materials
Year: 2021, Volume: 11, Issue: 4, Pages: 1-13 |
| ISSN: | 1614-6840 |
| DOI: | 10.1002/aenm.202002364 |
| Online Access: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1002/aenm.202002364 Verlag, lizenzpflichtig, Volltext: https://onlinelibrary.wiley.com/doi/abs/10.1002/aenm.202002364 
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| Author Notes: | Ruiyuan Tian, Aideen Griffin, Mark McCrystall, Madeleine Breshears, Andrew Harvey, Cian Gabbett, Dominik V. Horváth, Claudia Backes, Yu Jing, Thomas Heine, Sang-Hoon Park, João Coelho, Valeria Nicolosi, Markus Nentwig, Christopher Benndorf, Oliver Oeckler, and Jonathan N. Coleman |
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| 245 | 1 | 0 | |a Liquid exfoliated SnP3 nanosheets for very high areal capacity Lithium-Ion Batteries |c Ruiyuan Tian, Aideen Griffin, Mark McCrystall, Madeleine Breshears, Andrew Harvey, Cian Gabbett, Dominik V. Horváth, Claudia Backes, Yu Jing, Thomas Heine, Sang-Hoon Park, João Coelho, Valeria Nicolosi, Markus Nentwig, Christopher Benndorf, Oliver Oeckler, and Jonathan N. Coleman |
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| 500 | |a First published: 21 December 2020 | ||
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| 520 | |a Increasing the energy density of lithium-ion batteries requires the discovery of new electrode materials capable of achieving very high areal capacity. Here, liquid phase exfoliation is used to produce nanosheets of SnP3, a 2D material with extremely high theoretical capacity of 1670 mAh g−1. These nanosheets can be fabricated into solution-processed thin films for use as lithium storing anodes. To maximize their performance, carbon nanotubes are incorporated into the electrodes to simultaneously enhance conductivity and toughness. As a result, electrodes of thickness >300 µm can be produced, which display active-mass-normalized capacities (≈1657 mAh g−1Active) very close to the theoretical value. These materials show maximum specific (≈1250 mAh g−1Electrode) and areal (>20 mAh cm−2) capacities, which are at the state-of-the-art for 2D-based electrodes, coupled with good rate performance and stability. In combination with commercial cathode materials, full-cells are fabricated with areal capacities of ≈29 mAh cm−2 and near-record energy densities approaching 1000 Wh L−1. | ||
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