Molecular donor-acceptor dyads for efficient single-material organic solar cells
Single-material organic solar cells (SMOSCs) promise several advantages with respect to prospective applications in printed large-area solar foils. Only one photoactive material has to be processed and the impressive thermal and photochemical long-term stability of the devices is achieved. Herein, a...
Gespeichert in:
| Hauptverfasser: | , , , , , , , , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
Jan 2021
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| In: |
Solar RRL
Year: 2021, Jahrgang: 5, Heft: 1, Pages: 1-16 |
| ISSN: | 2367-198X |
| DOI: | 10.1002/solr.202000653 |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1002/solr.202000653 Verlag, lizenzpflichtig, Volltext: https://onlinelibrary.wiley.com/doi/abs/10.1002/solr.202000653 
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| Verfasserangaben: | Sebastian Lucas, Jochen Kammerer, Martin Pfannmöller, Rasmus R. Schröder, Yakun He, Ning Li, Christoph J. Brabec, Tim Leydecker, Paolo Samorì, Tomasz Marszalek, Wojchiech Pisula, Elena Mena-Osteritz, and Peter Bäuerle |
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| 245 | 1 | 0 | |a Molecular donor-acceptor dyads for efficient single-material organic solar cells |c Sebastian Lucas, Jochen Kammerer, Martin Pfannmöller, Rasmus R. Schröder, Yakun He, Ning Li, Christoph J. Brabec, Tim Leydecker, Paolo Samorì, Tomasz Marszalek, Wojchiech Pisula, Elena Mena-Osteritz, and Peter Bäuerle |
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| 500 | |a Gesehen am 22.03.2024 | ||
| 500 | |a Dedicated to Professor Franz Effenberger on the occasion of his 90th birthday | ||
| 520 | |a Single-material organic solar cells (SMOSCs) promise several advantages with respect to prospective applications in printed large-area solar foils. Only one photoactive material has to be processed and the impressive thermal and photochemical long-term stability of the devices is achieved. Herein, a novel structural design of oligomeric donor-acceptor (D-A) dyads 1-3 is established, in which an oligothiophene donor and fullerene acceptor are covalently linked by a flexible spacer of variable length. Favorable optoelectronic, charge transport, and self-organization properties of the D-A dyads are the basis for reaching power conversion efficiencies up to 4.26% in SMOSCs. The dependence of photovoltaic and charge transport parameters in these ambipolar semiconductors on the specific molecular structure is investigated before and after post-treatment by solvent vapor annealing. The inner nanomorphology of the photoactive films of the dyads is analyzed with transmission electron microscopy (TEM) and grazing-incidence wide-angle X-ray scattering (GIWAXS). Combined theoretical calculations result in a lamellar supramolecular order of the dyads with a D-A phase separation smaller than 2 nm. The molecular design and the precise distance between donor and acceptor moieties ensure the fundamental physical processes operative in organic solar cells and provide stabilization of D-A interfaces. | ||
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