Rebuilding the vibrational wavepacket in TRAS using attosecond X-ray pulses
Time-resolved X-ray photoelectron spectroscopy (TXPS) is a well-established technique to probe coherent nuclear wavepacket dynamics using both table-top and free-electron-based ultrafast X-ray lasers. Energy resolution, however, becomes compromised for a very short pulse duration in the sub-femtosec...
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| Main Authors: | , , , , , , , , , , |
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| Format: | Article (Journal) |
| Language: | English |
| Published: |
02 January 2024
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| In: |
Communications Physics
Year: 2024, Volume: 7, Issue: 1, Pages: 1-8 |
| ISSN: | 2399-3650 |
| DOI: | 10.1038/s42005-023-01507-3 |
| Online Access: | Verlag, kostenfrei, Volltext: https://doi.org/10.1038/s42005-023-01507-3 Verlag, kostenfrei, Volltext: https://www.nature.com/articles/s42005-023-01507-3 
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| Author Notes: | Chao Wang, Maomao Gong, Xi Zhao, Quan Wei Nan, Xin Yue Yu, Yongjun Cheng, Victor Kimberg, Xiao-Jing Liu, Oriol Vendrell, Kiyoshi Ueda and Song Bin Zhang |
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| 245 | 1 | 0 | |a Rebuilding the vibrational wavepacket in TRAS using attosecond X-ray pulses |c Chao Wang, Maomao Gong, Xi Zhao, Quan Wei Nan, Xin Yue Yu, Yongjun Cheng, Victor Kimberg, Xiao-Jing Liu, Oriol Vendrell, Kiyoshi Ueda and Song Bin Zhang |
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| 520 | |a Time-resolved X-ray photoelectron spectroscopy (TXPS) is a well-established technique to probe coherent nuclear wavepacket dynamics using both table-top and free-electron-based ultrafast X-ray lasers. Energy resolution, however, becomes compromised for a very short pulse duration in the sub-femtosecond range. By resonantly tuning the X-ray pulse to core-excited states undergoing Auger decay, this drawback of TXPS can be mitigated. While resonant Auger-electron spectroscopy (RAS) can recover the vibrational structures not hidden by broadband excitation, the full reconstruction of the wavepacket is a standing challenge. Here, we theoretically demonstrate how the complete information of a nuclear wavepacket, i.e., the populations and relative phases of the vibrational states constituting the wavepacket, can be retrieved from time-resolved RAS (TRAS) measurements. Thus, TRAS offers key insights into coupled nuclear and electronic dynamics in complex systems on ultrashort timescales, providing an alternative to leverage femtosecond and attosecond X-ray probe pulses. | ||
| 650 | 4 | |a Attosecond science | |
| 650 | 4 | |a Chemical physics | |
| 650 | 4 | |a Ultrafast photonics | |
| 650 | 4 | |a X-rays | |
| 700 | 1 | |a Gong, Maomao |e VerfasserIn |4 aut | |
| 700 | 1 | |a Zhao, Xi |e VerfasserIn |4 aut | |
| 700 | 1 | |a Nan, Quan Wei |e VerfasserIn |4 aut | |
| 700 | 1 | |a Yu, Xin Yue |e VerfasserIn |4 aut | |
| 700 | 1 | |a Cheng, Yongjun |e VerfasserIn |4 aut | |
| 700 | 1 | |a Kimberg, Victor |e VerfasserIn |4 aut | |
| 700 | 1 | |a Liu, Xiao-Jing |e VerfasserIn |4 aut | |
| 700 | 1 | |a Vendrell, Oriol |e VerfasserIn |0 (DE-588)1062512820 |0 (DE-627)80531511X |0 (DE-576)41827648X |4 aut | |
| 700 | 1 | |a Ueda, Kiyoshi |e VerfasserIn |4 aut | |
| 700 | 1 | |a Zhang, Song Bin |e VerfasserIn |4 aut | |
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