Emission control of entangled electrons in photoionisation of a hydrogen molecule

For photo-dissociation of a single hydrogen molecule ($$H_2$$) with combined XUV and IR laser pulses, we demonstrate optical control of the emission direction of the photoelectron with respect to the outgoing neutral fragment (the H-atom). Depending on the relative delay between the two laser fields...

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Hauptverfasser: Shobeiry, Farshad (VerfasserIn) , Froß, Patrick (VerfasserIn) , Srinivas, Hemkumar (VerfasserIn) , Pfeifer, Thomas (VerfasserIn) , Moshammer, Robert (VerfasserIn) , Harth, Anne (VerfasserIn)
Dokumenttyp: Article (Journal)
Sprache:Englisch
Veröffentlicht: 23 August 2024
In: Scientific reports
Year: 2024, Jahrgang: 14, Pages: 1-19
ISSN:2045-2322
DOI:10.1038/s41598-024-67465-0
Online-Zugang:Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1038/s41598-024-67465-0
Verlag, lizenzpflichtig, Volltext: https://www.nature.com/articles/s41598-024-67465-0
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Verfasserangaben:Farshad Shobeiry, Patrick Fross, Hemkumar Srinivas, Thomas Pfeifer, Robert Moshammer, Anne Harth
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Zusammenfassung:For photo-dissociation of a single hydrogen molecule ($$H_2$$) with combined XUV and IR laser pulses, we demonstrate optical control of the emission direction of the photoelectron with respect to the outgoing neutral fragment (the H-atom). Depending on the relative delay between the two laser fields, adjustable with sub-femtosecond time resolution, the photoelectron is emitted into the same hemisphere as the H-atom or opposite. This emission asymmetry is a result of entanglement of the two-electron final-state involving the spatially separated bound and emitted electron.
Beschreibung:Gesehen am 17.02.2025
Beschreibung:Online Resource
ISSN:2045-2322
DOI:10.1038/s41598-024-67465-0