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Controlling molecular dynamics by exciting atoms in a cavity

Placing an atom and a molecule in a cavity opens the door to initialize molecular dynamics by exciting a level of the atom. This approach enlarges the range of choosing the light source to trigger molecular dynamics substantially. The interplay of the atomic, molecular, and photonic populations give...

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Hauptverfasser: Csehi, András (VerfasserIn) , Szabó, Krisztián (VerfasserIn) , Vibók, Ágnes (VerfasserIn) , Cederbaum, Lorenz S. (VerfasserIn) , Halász, Gábor J. (VerfasserIn)
Dokumenttyp: Article (Journal)
Sprache:Englisch
Veröffentlicht: 5 May 2025
In: Physical review letters
Year: 2025, Jahrgang: 134, Heft: 18, Pages: 1-6
ISSN:1079-7114
DOI:10.1103/PhysRevLett.134.188001
Online-Zugang:Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1103/PhysRevLett.134.188001
Verlag, lizenzpflichtig, Volltext: https://link.aps.org/doi/10.1103/PhysRevLett.134.188001
Volltext
Verfasserangaben:András Csehi, Krisztián Szabó, Ágnes Vibók, Lorenz S. Cederbaum, and Gábor J. Halász

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520 |a Placing an atom and a molecule in a cavity opens the door to initialize molecular dynamics by exciting a level of the atom. This approach enlarges the range of choosing the light source to trigger molecular dynamics substantially. The interplay of the atomic, molecular, and photonic populations gives rise to rich dynamics. The cavity photon plays the role of a mediator between the atom and the molecule and it is found that the photonic population is rather low throughout and its evolution follows that of the molecule. Cavities are known to be subject to losses. In spite of the losses it is demonstrated that the presence of the atom gives rise to a long-lived dynamics that should be of relevance for experimental investigations. The presence of more atoms and molecules is expected to further enrich the dynamics. 
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