Site- and energy-selective low-energy electron emission by x-rays in the Aqueous Phase

Low-energy-electron emission from resonant Auger final states via intermolecular Coulombic decay (RA-ICD) has previously been described as a promising scenario for controlling radiation damage for medical purposes, but it has so far only been observed in prototypical atomic and molecular van der Waa...

Full description

Saved in:
Bibliographic Details
Main Authors: Bloß, Dana (Author) , Dupuy, Rémi (Author) , Trinter, Florian (Author) , Unger, Isaak (Author) , Walsh, Noelle (Author) , Öhrwall, Gunnar (Author) , Golchert, Niklas (Author) , Klassen, Gabriel (Author) , Krone, Adrian (Author) , Terao, Yusaku (Author) , Viehmann, Johannes H. (Author) , Wülfing, Lasse (Author) , Richter, Clemens (Author) , Buttersack, Tillmann (Author) , Cederbaum, Lorenz S. (Author) , Hergenhahn, Uwe (Author) , Björneholm, Olle (Author) , Ehresmann, Arno (Author) , Hans, Andreas (Author)
Format: Article (Journal)
Language:English
Published: 25 June 2025
In: Journal of the American Chemical Society
Year: 2025, Volume: 147, Issue: 25, Pages: 22115-22120
ISSN:1520-5126
DOI:10.1021/jacs.5c06436
Online Access:Verlag, kostenfrei, Volltext: https://doi.org/10.1021/jacs.5c06436
Get full text
Author Notes:Dana Bloß, Rémi Dupuy, Florian Trinter, Isaak Unger, Noelle Walsh, Gunnar Öhrwall, Niklas Golchert, Gabriel Klassen, Adrian Krone, Yusaku Terao, Johannes H. Viehmann, Lasse Wülfing, Clemens Richter, Tillmann Buttersack, Lorenz S. Cederbaum, Uwe Hergenhahn, Olle Björneholm, Arno Ehresmann, and Andreas Hans

MARC

LEADER 00000naa a2200000 c 4500
001 1939416507
003 DE-627
005 20251024122719.0
007 cr uuu---uuuuu
008 251024s2025 xx |||||o 00| ||eng c
024 7 |a 10.1021/jacs.5c06436  |2 doi 
035 |a (DE-627)1939416507 
035 |a (DE-599)KXP1939416507 
040 |a DE-627  |b ger  |c DE-627  |e rda 
041 |a eng 
084 |a 30  |2 sdnb 
100 1 |a Bloß, Dana  |e VerfasserIn  |0 (DE-588)1341435598  |0 (DE-627)1902191498  |4 aut 
245 1 0 |a Site- and energy-selective low-energy electron emission by x-rays in the Aqueous Phase  |c Dana Bloß, Rémi Dupuy, Florian Trinter, Isaak Unger, Noelle Walsh, Gunnar Öhrwall, Niklas Golchert, Gabriel Klassen, Adrian Krone, Yusaku Terao, Johannes H. Viehmann, Lasse Wülfing, Clemens Richter, Tillmann Buttersack, Lorenz S. Cederbaum, Uwe Hergenhahn, Olle Björneholm, Arno Ehresmann, and Andreas Hans 
264 1 |c 25 June 2025 
300 |b Illustrationen 
300 |a 6 
336 |a Text  |b txt  |2 rdacontent 
337 |a Computermedien  |b c  |2 rdamedia 
338 |a Online-Ressource  |b cr  |2 rdacarrier 
500 |a Online veröffentlicht: 13. Juni 2025 
500 |a Gesehen am 24.10.2025 
520 |a Low-energy-electron emission from resonant Auger final states via intermolecular Coulombic decay (RA-ICD) has previously been described as a promising scenario for controlling radiation damage for medical purposes, but it has so far only been observed in prototypical atomic and molecular van der Waals dimers and clusters. Here, we report the experimental observation of RA-ICD in an aqueous solution. We show that for solvated Ca2+ ions, the emission can be very efficiently controlled by tuning the photon energy of exciting X-rays to inner-shell resonances of the ions. Our results provide the next step from demonstrating RA-ICD in relatively simple prototype systems to understanding the relevance and potential applications of ICD in real-life scenarios. 
700 1 |a Dupuy, Rémi  |e VerfasserIn  |4 aut 
700 1 |a Trinter, Florian  |e VerfasserIn  |4 aut 
700 1 |a Unger, Isaak  |e VerfasserIn  |4 aut 
700 1 |a Walsh, Noelle  |e VerfasserIn  |4 aut 
700 1 |a Öhrwall, Gunnar  |e VerfasserIn  |4 aut 
700 1 |a Golchert, Niklas  |e VerfasserIn  |4 aut 
700 1 |a Klassen, Gabriel  |e VerfasserIn  |4 aut 
700 1 |a Krone, Adrian  |e VerfasserIn  |4 aut 
700 1 |a Terao, Yusaku  |e VerfasserIn  |4 aut 
700 1 |a Viehmann, Johannes H.  |e VerfasserIn  |4 aut 
700 1 |a Wülfing, Lasse  |e VerfasserIn  |4 aut 
700 1 |a Richter, Clemens  |e VerfasserIn  |4 aut 
700 1 |a Buttersack, Tillmann  |e VerfasserIn  |4 aut 
700 1 |a Cederbaum, Lorenz S.  |d 1946-  |e VerfasserIn  |0 (DE-588)172484952  |0 (DE-627)697422798  |0 (DE-576)133346145  |4 aut 
700 1 |a Hergenhahn, Uwe  |e VerfasserIn  |4 aut 
700 1 |a Björneholm, Olle  |e VerfasserIn  |4 aut 
700 1 |a Ehresmann, Arno  |e VerfasserIn  |4 aut 
700 1 |a Hans, Andreas  |e VerfasserIn  |4 aut 
773 0 8 |i Enthalten in  |a American Chemical Society  |t Journal of the American Chemical Society  |d Washington, DC : ACS Publications, 1879  |g 147(2025), 25 vom: Juni, Seite 22115-22120  |w (DE-627)268132836  |w (DE-600)1472210-0  |w (DE-576)090854284  |x 1520-5126  |7 nnas 
773 1 8 |g volume:147  |g year:2025  |g number:25  |g month:06  |g pages:22115-22120  |g extent:6  |a Site- and energy-selective low-energy electron emission by x-rays in the Aqueous Phase 
856 4 0 |u https://doi.org/10.1021/jacs.5c06436  |x Verlag  |x Resolving-System  |z kostenfrei  |3 Volltext 
951 |a AR 
992 |a 20251024 
993 |a Article 
994 |a 2025 
998 |g 172484952  |a Cederbaum, Lorenz S.  |m 172484952:Cederbaum, Lorenz S.  |d 120000  |d 120300  |e 120000PC172484952  |e 120300PC172484952  |k 0/120000/  |k 1/120000/120300/  |p 15 
999 |a KXP-PPN1939416507  |e 4791465407 
BIB |a Y 
SER |a journal 
JSO |a {"title":[{"title":"Site- and energy-selective low-energy electron emission by x-rays in the Aqueous Phase","title_sort":"Site- and energy-selective low-energy electron emission by x-rays in the Aqueous Phase"}],"physDesc":[{"extent":"6 S.","noteIll":"Illustrationen"}],"person":[{"family":"Bloß","given":"Dana","roleDisplay":"VerfasserIn","display":"Bloß, Dana","role":"aut"},{"role":"aut","display":"Dupuy, Rémi","roleDisplay":"VerfasserIn","given":"Rémi","family":"Dupuy"},{"family":"Trinter","roleDisplay":"VerfasserIn","given":"Florian","display":"Trinter, Florian","role":"aut"},{"roleDisplay":"VerfasserIn","given":"Isaak","family":"Unger","role":"aut","display":"Unger, Isaak"},{"display":"Walsh, Noelle","role":"aut","family":"Walsh","given":"Noelle","roleDisplay":"VerfasserIn"},{"role":"aut","display":"Öhrwall, Gunnar","roleDisplay":"VerfasserIn","given":"Gunnar","family":"Öhrwall"},{"display":"Golchert, Niklas","role":"aut","family":"Golchert","given":"Niklas","roleDisplay":"VerfasserIn"},{"role":"aut","display":"Klassen, Gabriel","given":"Gabriel","roleDisplay":"VerfasserIn","family":"Klassen"},{"roleDisplay":"VerfasserIn","given":"Adrian","family":"Krone","role":"aut","display":"Krone, Adrian"},{"display":"Terao, Yusaku","role":"aut","family":"Terao","roleDisplay":"VerfasserIn","given":"Yusaku"},{"given":"Johannes H.","roleDisplay":"VerfasserIn","family":"Viehmann","role":"aut","display":"Viehmann, Johannes H."},{"family":"Wülfing","given":"Lasse","roleDisplay":"VerfasserIn","display":"Wülfing, Lasse","role":"aut"},{"role":"aut","display":"Richter, Clemens","given":"Clemens","roleDisplay":"VerfasserIn","family":"Richter"},{"family":"Buttersack","roleDisplay":"VerfasserIn","given":"Tillmann","display":"Buttersack, Tillmann","role":"aut"},{"display":"Cederbaum, Lorenz S.","role":"aut","family":"Cederbaum","given":"Lorenz S.","roleDisplay":"VerfasserIn"},{"family":"Hergenhahn","roleDisplay":"VerfasserIn","given":"Uwe","display":"Hergenhahn, Uwe","role":"aut"},{"given":"Olle","roleDisplay":"VerfasserIn","family":"Björneholm","role":"aut","display":"Björneholm, Olle"},{"family":"Ehresmann","given":"Arno","roleDisplay":"VerfasserIn","display":"Ehresmann, Arno","role":"aut"},{"role":"aut","display":"Hans, Andreas","given":"Andreas","roleDisplay":"VerfasserIn","family":"Hans"}],"relHost":[{"recId":"268132836","disp":"American Chemical SocietyJournal of the American Chemical Society","title":[{"title_sort":"Journal of the American Chemical Society","subtitle":"JACS","title":"Journal of the American Chemical Society"}],"corporate":[{"display":"American Chemical Society","role":"aut","roleDisplay":"VerfasserIn"}],"name":{"displayForm":["Ed.: Allen J. Bard [u.a.]"]},"note":["Gesehen am 25.08.2020"],"titleAlt":[{"title":"JACS"},{"title":"web edition"}],"id":{"issn":["1520-5126"],"eki":["268132836"],"zdb":["1472210-0"]},"type":{"bibl":"periodical","media":"Online-Ressource"},"origin":[{"publisherPlace":"Washington, DC ; Washington, DC","dateIssuedKey":"1879","publisher":"ACS Publications ; American Chemical Society","dateIssuedDisp":"1879-"}],"part":{"year":"2025","volume":"147","text":"147(2025), 25 vom: Juni, Seite 22115-22120","issue":"25","pages":"22115-22120","extent":"6"},"pubHistory":["1.1879 -"],"language":["eng"]}],"name":{"displayForm":["Dana Bloß, Rémi Dupuy, Florian Trinter, Isaak Unger, Noelle Walsh, Gunnar Öhrwall, Niklas Golchert, Gabriel Klassen, Adrian Krone, Yusaku Terao, Johannes H. Viehmann, Lasse Wülfing, Clemens Richter, Tillmann Buttersack, Lorenz S. Cederbaum, Uwe Hergenhahn, Olle Björneholm, Arno Ehresmann, and Andreas Hans"]},"note":["Online veröffentlicht: 13. Juni 2025","Gesehen am 24.10.2025"],"id":{"doi":["10.1021/jacs.5c06436"],"eki":["1939416507"]},"language":["eng"],"recId":"1939416507","type":{"media":"Online-Ressource","bibl":"article-journal"},"origin":[{"dateIssuedKey":"2025","dateIssuedDisp":"25 June 2025"}]} 
SRT |a BLOSSDANADSITEANDENE2520