Site- and energy-selective low-energy electron emission by x-rays in the Aqueous Phase
Low-energy-electron emission from resonant Auger final states via intermolecular Coulombic decay (RA-ICD) has previously been described as a promising scenario for controlling radiation damage for medical purposes, but it has so far only been observed in prototypical atomic and molecular van der Waa...
Saved in:
| Main Authors: | , , , , , , , , , , , , , , , , , , |
|---|---|
| Format: | Article (Journal) |
| Language: | English |
| Published: |
25 June 2025
|
| In: |
Journal of the American Chemical Society
Year: 2025, Volume: 147, Issue: 25, Pages: 22115-22120 |
| ISSN: | 1520-5126 |
| DOI: | 10.1021/jacs.5c06436 |
| Online Access: | Verlag, kostenfrei, Volltext: https://doi.org/10.1021/jacs.5c06436 |
| Author Notes: | Dana Bloß, Rémi Dupuy, Florian Trinter, Isaak Unger, Noelle Walsh, Gunnar Öhrwall, Niklas Golchert, Gabriel Klassen, Adrian Krone, Yusaku Terao, Johannes H. Viehmann, Lasse Wülfing, Clemens Richter, Tillmann Buttersack, Lorenz S. Cederbaum, Uwe Hergenhahn, Olle Björneholm, Arno Ehresmann, and Andreas Hans |
MARC
| LEADER | 00000naa a2200000 c 4500 | ||
|---|---|---|---|
| 001 | 1939416507 | ||
| 003 | DE-627 | ||
| 005 | 20251024122719.0 | ||
| 007 | cr uuu---uuuuu | ||
| 008 | 251024s2025 xx |||||o 00| ||eng c | ||
| 024 | 7 | |a 10.1021/jacs.5c06436 |2 doi | |
| 035 | |a (DE-627)1939416507 | ||
| 035 | |a (DE-599)KXP1939416507 | ||
| 040 | |a DE-627 |b ger |c DE-627 |e rda | ||
| 041 | |a eng | ||
| 084 | |a 30 |2 sdnb | ||
| 100 | 1 | |a Bloß, Dana |e VerfasserIn |0 (DE-588)1341435598 |0 (DE-627)1902191498 |4 aut | |
| 245 | 1 | 0 | |a Site- and energy-selective low-energy electron emission by x-rays in the Aqueous Phase |c Dana Bloß, Rémi Dupuy, Florian Trinter, Isaak Unger, Noelle Walsh, Gunnar Öhrwall, Niklas Golchert, Gabriel Klassen, Adrian Krone, Yusaku Terao, Johannes H. Viehmann, Lasse Wülfing, Clemens Richter, Tillmann Buttersack, Lorenz S. Cederbaum, Uwe Hergenhahn, Olle Björneholm, Arno Ehresmann, and Andreas Hans |
| 264 | 1 | |c 25 June 2025 | |
| 300 | |b Illustrationen | ||
| 300 | |a 6 | ||
| 336 | |a Text |b txt |2 rdacontent | ||
| 337 | |a Computermedien |b c |2 rdamedia | ||
| 338 | |a Online-Ressource |b cr |2 rdacarrier | ||
| 500 | |a Online veröffentlicht: 13. Juni 2025 | ||
| 500 | |a Gesehen am 24.10.2025 | ||
| 520 | |a Low-energy-electron emission from resonant Auger final states via intermolecular Coulombic decay (RA-ICD) has previously been described as a promising scenario for controlling radiation damage for medical purposes, but it has so far only been observed in prototypical atomic and molecular van der Waals dimers and clusters. Here, we report the experimental observation of RA-ICD in an aqueous solution. We show that for solvated Ca2+ ions, the emission can be very efficiently controlled by tuning the photon energy of exciting X-rays to inner-shell resonances of the ions. Our results provide the next step from demonstrating RA-ICD in relatively simple prototype systems to understanding the relevance and potential applications of ICD in real-life scenarios. | ||
| 700 | 1 | |a Dupuy, Rémi |e VerfasserIn |4 aut | |
| 700 | 1 | |a Trinter, Florian |e VerfasserIn |4 aut | |
| 700 | 1 | |a Unger, Isaak |e VerfasserIn |4 aut | |
| 700 | 1 | |a Walsh, Noelle |e VerfasserIn |4 aut | |
| 700 | 1 | |a Öhrwall, Gunnar |e VerfasserIn |4 aut | |
| 700 | 1 | |a Golchert, Niklas |e VerfasserIn |4 aut | |
| 700 | 1 | |a Klassen, Gabriel |e VerfasserIn |4 aut | |
| 700 | 1 | |a Krone, Adrian |e VerfasserIn |4 aut | |
| 700 | 1 | |a Terao, Yusaku |e VerfasserIn |4 aut | |
| 700 | 1 | |a Viehmann, Johannes H. |e VerfasserIn |4 aut | |
| 700 | 1 | |a Wülfing, Lasse |e VerfasserIn |4 aut | |
| 700 | 1 | |a Richter, Clemens |e VerfasserIn |4 aut | |
| 700 | 1 | |a Buttersack, Tillmann |e VerfasserIn |4 aut | |
| 700 | 1 | |a Cederbaum, Lorenz S. |d 1946- |e VerfasserIn |0 (DE-588)172484952 |0 (DE-627)697422798 |0 (DE-576)133346145 |4 aut | |
| 700 | 1 | |a Hergenhahn, Uwe |e VerfasserIn |4 aut | |
| 700 | 1 | |a Björneholm, Olle |e VerfasserIn |4 aut | |
| 700 | 1 | |a Ehresmann, Arno |e VerfasserIn |4 aut | |
| 700 | 1 | |a Hans, Andreas |e VerfasserIn |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |a American Chemical Society |t Journal of the American Chemical Society |d Washington, DC : ACS Publications, 1879 |g 147(2025), 25 vom: Juni, Seite 22115-22120 |w (DE-627)268132836 |w (DE-600)1472210-0 |w (DE-576)090854284 |x 1520-5126 |7 nnas |
| 773 | 1 | 8 | |g volume:147 |g year:2025 |g number:25 |g month:06 |g pages:22115-22120 |g extent:6 |a Site- and energy-selective low-energy electron emission by x-rays in the Aqueous Phase |
| 856 | 4 | 0 | |u https://doi.org/10.1021/jacs.5c06436 |x Verlag |x Resolving-System |z kostenfrei |3 Volltext |
| 951 | |a AR | ||
| 992 | |a 20251024 | ||
| 993 | |a Article | ||
| 994 | |a 2025 | ||
| 998 | |g 172484952 |a Cederbaum, Lorenz S. |m 172484952:Cederbaum, Lorenz S. |d 120000 |d 120300 |e 120000PC172484952 |e 120300PC172484952 |k 0/120000/ |k 1/120000/120300/ |p 15 | ||
| 999 | |a KXP-PPN1939416507 |e 4791465407 | ||
| BIB | |a Y | ||
| SER | |a journal | ||
| JSO | |a {"title":[{"title":"Site- and energy-selective low-energy electron emission by x-rays in the Aqueous Phase","title_sort":"Site- and energy-selective low-energy electron emission by x-rays in the Aqueous Phase"}],"physDesc":[{"extent":"6 S.","noteIll":"Illustrationen"}],"person":[{"family":"Bloß","given":"Dana","roleDisplay":"VerfasserIn","display":"Bloß, Dana","role":"aut"},{"role":"aut","display":"Dupuy, Rémi","roleDisplay":"VerfasserIn","given":"Rémi","family":"Dupuy"},{"family":"Trinter","roleDisplay":"VerfasserIn","given":"Florian","display":"Trinter, Florian","role":"aut"},{"roleDisplay":"VerfasserIn","given":"Isaak","family":"Unger","role":"aut","display":"Unger, Isaak"},{"display":"Walsh, Noelle","role":"aut","family":"Walsh","given":"Noelle","roleDisplay":"VerfasserIn"},{"role":"aut","display":"Öhrwall, Gunnar","roleDisplay":"VerfasserIn","given":"Gunnar","family":"Öhrwall"},{"display":"Golchert, Niklas","role":"aut","family":"Golchert","given":"Niklas","roleDisplay":"VerfasserIn"},{"role":"aut","display":"Klassen, Gabriel","given":"Gabriel","roleDisplay":"VerfasserIn","family":"Klassen"},{"roleDisplay":"VerfasserIn","given":"Adrian","family":"Krone","role":"aut","display":"Krone, Adrian"},{"display":"Terao, Yusaku","role":"aut","family":"Terao","roleDisplay":"VerfasserIn","given":"Yusaku"},{"given":"Johannes H.","roleDisplay":"VerfasserIn","family":"Viehmann","role":"aut","display":"Viehmann, Johannes H."},{"family":"Wülfing","given":"Lasse","roleDisplay":"VerfasserIn","display":"Wülfing, Lasse","role":"aut"},{"role":"aut","display":"Richter, Clemens","given":"Clemens","roleDisplay":"VerfasserIn","family":"Richter"},{"family":"Buttersack","roleDisplay":"VerfasserIn","given":"Tillmann","display":"Buttersack, Tillmann","role":"aut"},{"display":"Cederbaum, Lorenz S.","role":"aut","family":"Cederbaum","given":"Lorenz S.","roleDisplay":"VerfasserIn"},{"family":"Hergenhahn","roleDisplay":"VerfasserIn","given":"Uwe","display":"Hergenhahn, Uwe","role":"aut"},{"given":"Olle","roleDisplay":"VerfasserIn","family":"Björneholm","role":"aut","display":"Björneholm, Olle"},{"family":"Ehresmann","given":"Arno","roleDisplay":"VerfasserIn","display":"Ehresmann, Arno","role":"aut"},{"role":"aut","display":"Hans, Andreas","given":"Andreas","roleDisplay":"VerfasserIn","family":"Hans"}],"relHost":[{"recId":"268132836","disp":"American Chemical SocietyJournal of the American Chemical Society","title":[{"title_sort":"Journal of the American Chemical Society","subtitle":"JACS","title":"Journal of the American Chemical Society"}],"corporate":[{"display":"American Chemical Society","role":"aut","roleDisplay":"VerfasserIn"}],"name":{"displayForm":["Ed.: Allen J. Bard [u.a.]"]},"note":["Gesehen am 25.08.2020"],"titleAlt":[{"title":"JACS"},{"title":"web edition"}],"id":{"issn":["1520-5126"],"eki":["268132836"],"zdb":["1472210-0"]},"type":{"bibl":"periodical","media":"Online-Ressource"},"origin":[{"publisherPlace":"Washington, DC ; Washington, DC","dateIssuedKey":"1879","publisher":"ACS Publications ; American Chemical Society","dateIssuedDisp":"1879-"}],"part":{"year":"2025","volume":"147","text":"147(2025), 25 vom: Juni, Seite 22115-22120","issue":"25","pages":"22115-22120","extent":"6"},"pubHistory":["1.1879 -"],"language":["eng"]}],"name":{"displayForm":["Dana Bloß, Rémi Dupuy, Florian Trinter, Isaak Unger, Noelle Walsh, Gunnar Öhrwall, Niklas Golchert, Gabriel Klassen, Adrian Krone, Yusaku Terao, Johannes H. Viehmann, Lasse Wülfing, Clemens Richter, Tillmann Buttersack, Lorenz S. Cederbaum, Uwe Hergenhahn, Olle Björneholm, Arno Ehresmann, and Andreas Hans"]},"note":["Online veröffentlicht: 13. Juni 2025","Gesehen am 24.10.2025"],"id":{"doi":["10.1021/jacs.5c06436"],"eki":["1939416507"]},"language":["eng"],"recId":"1939416507","type":{"media":"Online-Ressource","bibl":"article-journal"},"origin":[{"dateIssuedKey":"2025","dateIssuedDisp":"25 June 2025"}]} | ||
| SRT | |a BLOSSDANADSITEANDENE2520 | ||