Quantum dynamics simulation of exciton-polariton transport
Abstract - Strong coupling between excitons and confined modes of light presents a promising pathway to tunable and enhanced energy transport in organic materials. By forming hybrid light-matter quasiparticles, exciton-polaritons, electronic excitations can traverse long distances at high velocities...
Gespeichert in:
| Hauptverfasser: | , , |
|---|---|
| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
01 July 2025
|
| In: |
Nature Communications
Year: 2025, Jahrgang: 16, Pages: 1-12 |
| ISSN: | 2041-1723 |
| DOI: | 10.1038/s41467-025-61298-9 |
| Online-Zugang: | Verlag, kostenfrei, Volltext: https://doi.org/10.1038/s41467-025-61298-9 Verlag, kostenfrei, Volltext: https://www.nature.com/articles/s41467-025-61298-9 
|
| Verfasserangaben: | Niclas Krupp, Gerrit Groenhof Oriol & Vendrell |
MARC
| LEADER | 00000caa a2200000 c 4500 | ||
|---|---|---|---|
| 001 | 1942140444 | ||
| 003 | DE-627 | ||
| 005 | 20251126150255.0 | ||
| 007 | cr uuu---uuuuu | ||
| 008 | 251124s2025 xx |||||o 00| ||eng c | ||
| 024 | 7 | |a 10.1038/s41467-025-61298-9 |2 doi | |
| 035 | |a (DE-627)1942140444 | ||
| 035 | |a (DE-599)KXP1942140444 | ||
| 040 | |a DE-627 |b ger |c DE-627 |e rda | ||
| 041 | |a eng | ||
| 084 | |a 29 |2 sdnb | ||
| 100 | 1 | |a Krupp, Niclas |e VerfasserIn |0 (DE-588)1382432771 |0 (DE-627)1942141939 |4 aut | |
| 245 | 1 | 0 | |a Quantum dynamics simulation of exciton-polariton transport |c Niclas Krupp, Gerrit Groenhof Oriol & Vendrell |
| 264 | 1 | |c 01 July 2025 | |
| 300 | |a 12 | ||
| 336 | |a Text |b txt |2 rdacontent | ||
| 337 | |a Computermedien |b c |2 rdamedia | ||
| 338 | |a Online-Ressource |b cr |2 rdacarrier | ||
| 500 | |a Gesehen am 24.11.2025 | ||
| 520 | |a Abstract - Strong coupling between excitons and confined modes of light presents a promising pathway to tunable and enhanced energy transport in organic materials. By forming hybrid light-matter quasiparticles, exciton-polaritons, electronic excitations can traverse long distances at high velocities through ballistic flow. However, transport behavior of exciton-polaritons varies strongly across experiments, spanning both diffusive and ballistic transport regimes. Which properties of the material and light-modes govern the transport behavior of polaritons remains an open question. Through full-quantum dynamical simulations we reveal a strong dependence of polariton transport on vibronic interactions and static disorder within molecules in both ideal and lossy cavities. Specifically, we show that intramolecular vibrations mediate relaxation processes that alter polariton composition, lifetime and velocity on ultrafast timescales. Analysis of the propagating wavepacket in position and momentum space provides mechanistic insight into the robustness of ballistic flow of exciton-polaritons found experimentally under cryogenic conditions. | ||
| 700 | 1 | |a Groenhof, Gerrit |e VerfasserIn |0 (DE-588)1382433166 |0 (DE-627)1942145616 |4 aut | |
| 700 | 1 | |a Vendrell, Oriol |e VerfasserIn |0 (DE-588)1062512820 |0 (DE-627)80531511X |0 (DE-576)41827648X |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Nature Communications |d [London] : Springer Nature, 2010 |g 16(2025), Artikel-ID 5431, Seite 1-12 |h Online-Ressource |w (DE-627)626457688 |w (DE-600)2553671-0 |w (DE-576)331555905 |x 2041-1723 |7 nnas |a Quantum dynamics simulation of exciton-polariton transport |
| 773 | 1 | 8 | |g volume:16 |g year:2025 |g elocationid:5431 |g pages:1-12 |g extent:12 |a Quantum dynamics simulation of exciton-polariton transport |
| 856 | 4 | 0 | |u https://doi.org/10.1038/s41467-025-61298-9 |x Verlag |x Resolving-System |z kostenfrei |3 Volltext |
| 856 | 4 | 0 | |u https://www.nature.com/articles/s41467-025-61298-9 |x Verlag |z kostenfrei |3 Volltext |
| 951 | |a AR | ||
| 992 | |a 20251124 | ||
| 993 | |a Article | ||
| 994 | |a 2025 | ||
| 998 | |g 1062512820 |a Vendrell, Oriol |m 1062512820:Vendrell, Oriol |d 120000 |d 120300 |e 120000PV1062512820 |e 120300PV1062512820 |k 0/120000/ |k 1/120000/120300/ |p 3 |y j | ||
| 998 | |g 1382432771 |a Krupp, Niclas |m 1382432771:Krupp, Niclas |d 120000 |d 120300 |e 120000PK1382432771 |e 120300PK1382432771 |k 0/120000/ |k 1/120000/120300/ |p 1 |x j | ||
| 999 | |a KXP-PPN1942140444 |e 481211067X | ||
| BIB | |a Y | ||
| SER | |a journal | ||
| JSO | |a {"note":["Gesehen am 24.11.2025"],"id":{"eki":["1942140444"],"doi":["10.1038/s41467-025-61298-9"]},"title":[{"title":"Quantum dynamics simulation of exciton-polariton transport","title_sort":"Quantum dynamics simulation of exciton-polariton transport"}],"recId":"1942140444","relHost":[{"disp":"Quantum dynamics simulation of exciton-polariton transportNature Communications","note":["Gesehen am 13.06.24"],"title":[{"title":"Nature Communications","title_sort":"Nature Communications"}],"id":{"issn":["2041-1723"],"eki":["626457688"],"zdb":["2553671-0"]},"physDesc":[{"extent":"Online-Ressource"}],"part":{"pages":"1-12","year":"2025","extent":"12","volume":"16","text":"16(2025), Artikel-ID 5431, Seite 1-12"},"type":{"media":"Online-Ressource","bibl":"periodical"},"origin":[{"publisherPlace":"[London] ; [London]","dateIssuedDisp":"[2010]-","publisher":"Springer Nature ; Nature Publishing Group UK"}],"language":["eng"],"pubHistory":["2010-"],"recId":"626457688"}],"person":[{"family":"Krupp","roleDisplay":"VerfasserIn","role":"aut","display":"Krupp, Niclas","given":"Niclas"},{"family":"Groenhof","roleDisplay":"VerfasserIn","given":"Gerrit","display":"Groenhof, Gerrit","role":"aut"},{"roleDisplay":"VerfasserIn","family":"Vendrell","role":"aut","display":"Vendrell, Oriol","given":"Oriol"}],"name":{"displayForm":["Niclas Krupp, Gerrit Groenhof Oriol & Vendrell"]},"physDesc":[{"extent":"12 S."}],"language":["eng"],"type":{"media":"Online-Ressource","bibl":"article-journal"},"origin":[{"dateIssuedKey":"2025","dateIssuedDisp":"01 July 2025"}]} | ||
| SRT | |a KRUPPNICLAQUANTUMDYN0120 | ||