A preorganized triarmed bis-triazolylpyridine-calix(4)arene with high affinity and selectivity for minor actinides for nuclear waste treatment
The incorporation of three terdentate 2,6-bis-triazolyl-pyridine units on a calix[4]arene gives a preorganized lipophilic ligand with enhanced efficiency in binding trivalent actinides over lanthanides. Combined time-resolved laser-induced fluorescence spectroscopy, and 1D and 1H-15N HMQC NMR invest...
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| Hauptverfasser: | , , , , , , , , , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
13 Aug 2025
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| In: |
Chemical communications
Year: 2025, Jahrgang: 61, Heft: 73, Pages: 13968-13971 |
| ISSN: | 1364-548X |
| DOI: | 10.1039/D5CC02948A |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1039/D5CC02948A Verlag, lizenzpflichtig, Volltext: https://pubs.rsc.org/en/content/articlelanding/2025/cc/d5cc02948a 
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| Verfasserangaben: | Davide Baccelli, Jonas Stracke, Maria Chiara Gullo, Patrik Weßling, Symeon Grivas, Francesco Rispoli, Stefano Volpi, Andrea Mele, Andreas Geist, Petra J. Panak, Francesco Sansone, Thomas Sittel, Elena Macerata and Alessandro Casnati |
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| 520 | |a The incorporation of three terdentate 2,6-bis-triazolyl-pyridine units on a calix[4]arene gives a preorganized lipophilic ligand with enhanced efficiency in binding trivalent actinides over lanthanides. Combined time-resolved laser-induced fluorescence spectroscopy, and 1D and 1H-15N HMQC NMR investigations allowed to propose the structures of the complexes and to provide insights into the actinide selectivity. | ||
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