Electronic and spin states of SrRuO 3 thin films: an x-ray magnetic circular dichroism study

We report a study of the local magnetism in thin films of SrRuO3 grown on (111) and (001) oriented SrTiO3 substrates using x-ray magnetic circular dichroism spectroscopy (XMCD) at the Ru-L2,3 edges. The application of the sum rules to the XMCD data gives an almost quenched orbital moment and a spin...

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Main Authors: Agrestini, Stefano (Author) , Hu, Zhimin (Author) , Haverkort, Maurits W. (Author)
Format: Article (Journal)
Language:English
Published: 24 February 2015
In: Physical review. B, Condensed matter and materials physics
Year: 2015, Volume: 91, Issue: 7, Pages: 075127
ISSN:1550-235X
DOI:10.1103/PhysRevB.91.075127
Online Access:Verlag, Volltext: http://dx.doi.org/10.1103/PhysRevB.91.075127
Verlag, Volltext: https://link.aps.org/doi/10.1103/PhysRevB.91.075127
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Author Notes:S. Agrestini, Z. Hu, C.-Y. Kuo, M.W. Haverkort, K.-T. Ko, N. Hollmann, Q. Liu, E. Pellegrin, M. Valvidares, J. Herrero-Martin, P. Gargiani, P. Gegenwart, M. Schneider, S. Esser, A. Tanaka, A.C. Komarek, and L.H. Tjeng
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Summary:We report a study of the local magnetism in thin films of SrRuO3 grown on (111) and (001) oriented SrTiO3 substrates using x-ray magnetic circular dichroism spectroscopy (XMCD) at the Ru-L2,3 edges. The application of the sum rules to the XMCD data gives an almost quenched orbital moment and a spin moment close to the value expected for the low spin state S=1. Full-multiplet cluster calculations indicate that the low spin state is quite stable and suggest that the occurrence of a transition to the high spin state S=2 in strained thin films of SrRuO3 is unlikely as it would be too expensive in energy.
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Physical Description:Online Resource
ISSN:1550-235X
DOI:10.1103/PhysRevB.91.075127