The combination of Benzaldehyde and Nickel‐catalyzed photoredox C(sp3)-H alkylation/arylation
Herein we report a highly selective photoredox C(sp3)−H alkylation/arylation of ethers through the combination of a photo‐organocatalyst (benzaldehyde) and a transition‐metal catalyst (nickel). This method provides a simple and general strategy for the C(sp3)−H alkylation/arylation of ethers. A sele...
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| Hauptverfasser: | , , , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Deutsch |
| Veröffentlicht: |
January 9, 2019
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| In: |
Angewandte Chemie. International edition
Year: 2019, Jahrgang: 58, Heft: 6, Pages: 1823-1827 |
| ISSN: | 1521-3773 |
| DOI: | 10.1002/anie.201810526 |
| Online-Zugang: | Resolving-System, Volltext: http://dx.doi.org/10.1002/anie.201810526 Verlag, Volltext: https://onlinelibrary.wiley.com/doi/abs/10.1002/anie.201810526 
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| Verfasserangaben: | Lumin Zhang, Xiaojia Si, Yangyang Yang, Marc Zimmer, Sina Witzel, Kohei Sekine, Matthias Rudolph, and A. Stephen K. Hashmi |
MARC
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| 245 | 1 | 0 | |a The combination of Benzaldehyde and Nickel‐catalyzed photoredox C(sp3)-H alkylation/arylation |c Lumin Zhang, Xiaojia Si, Yangyang Yang, Marc Zimmer, Sina Witzel, Kohei Sekine, Matthias Rudolph, and A. Stephen K. Hashmi |
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| 520 | |a Herein we report a highly selective photoredox C(sp3)−H alkylation/arylation of ethers through the combination of a photo‐organocatalyst (benzaldehyde) and a transition‐metal catalyst (nickel). This method provides a simple and general strategy for the C(sp3)−H alkylation/arylation of ethers. A selective late‐stage modification of (−)‐ambroxide has also been conducted to demonstrate the applicability of the method. | ||
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