Electron correlation driven non-adiabatic relaxation in molecules excited by an ultrashort extreme ultraviolet pulse

The many-body quantum nature of molecules determines their static and dynamic properties, but remains the main obstacle in their accurate description. Here, the authors employ ultrafast spectroscopic methods to explore the dynamics of highly excited organic molecules, revealing many-body effects and...

Full description

Saved in:
Bibliographic Details
Main Authors: Marciniak, Alexandre (Author) , Despré, Victor (Author) , Kuleff, Alexander I. (Author)
Format: Article (Journal)
Language:English
Published: 18 January 2019
In: Nature Communications
Year: 2019, Volume: 10
ISSN:2041-1723
DOI:10.1038/s41467-018-08131-8
Online Access:Verlag, Volltext: http://dx.doi.org/10.1038/s41467-018-08131-8
Verlag, Volltext: https://www.nature.com/articles/s41467-018-08131-8
Get full text
Author Notes:A. Marciniak, V. Despré, V. Loriot, G. Karras, M. Hervé, L. Quintard, F. Catoire, C. Joblin, E. Constant, A.I. Kuleff & F. Lépine
Description
Summary:The many-body quantum nature of molecules determines their static and dynamic properties, but remains the main obstacle in their accurate description. Here, the authors employ ultrafast spectroscopic methods to explore the dynamics of highly excited organic molecules, revealing many-body effects and hints of coherent vibronic dynamics which persist despite their molecular complexity.
Item Description:Gesehen am 06.03.2019
Physical Description:Online Resource
ISSN:2041-1723
DOI:10.1038/s41467-018-08131-8