Rapid multiple-quantum three-dimensional fluorescence spectroscopy disentangles quantum pathways

Multidimensional spectroscopic tools are important to explore the details of molecular dynamics. Here the authors use shaped pulses to demonstrate a 3D fluorescence spectroscopy method to extract the fourth and higher-order nonlinear responses in light-molecule interaction.

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Bibliographic Details
Main Authors: Müller, Stefan (Author) , Lüttig, Julian (Author) , Malý, Pavel (Author) , Ji, Lei (Author) , Han, Jie (Author) , Moos, Michael (Author) , Marder, Todd B. (Author) , Bunz, Uwe H. F. (Author) , Dreuw, Andreas (Author) , Lambert, Christoph (Author) , Brixner, Tobias (Author)
Format: Article (Journal)
Language:English
Published: 18 October 2019
In: Nature Communications
Year: 2019, Volume: 10
ISSN:2041-1723
DOI:10.1038/s41467-019-12602-x
Online Access:Verlag, Volltext: https://doi.org/10.1038/s41467-019-12602-x
Verlag, Volltext: https://www.nature.com/articles/s41467-019-12602-x
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Author Notes:Stefan Mueller, Julian Lüttig, Pavel Malý, Lei Ji, Jie Han, Michael Moos, Todd B. Marder, Uwe H.F. Bunz, Andreas Dreuw, Christoph Lambert &Tobias Brixner
Description
Summary:Multidimensional spectroscopic tools are important to explore the details of molecular dynamics. Here the authors use shaped pulses to demonstrate a 3D fluorescence spectroscopy method to extract the fourth and higher-order nonlinear responses in light-molecule interaction.
Item Description:Gesehen am 14.01.2020
Physical Description:Online Resource
ISSN:2041-1723
DOI:10.1038/s41467-019-12602-x