Population redistribution in optically trapped polar molecules
We investigate the rovibrational population redistribution of polar molecules in theelectronic ground state induced by spontaneous emission and blackbody radiation. As amodel system we use optically trapped LiCs molecules formed by photoassociation in anultracold two-species gas. The population dyna...
Saved in:
| Main Authors: | , , , , |
|---|---|
| Format: | Article (Journal) |
| Language: | English |
| Published: |
19 September 2011
|
| In: |
The European physical journal. D, Atomic, molecular, optical and plasma physics
Year: 2011, Volume: 65, Pages: 99-104 |
| ISSN: | 1434-6079 |
| DOI: | 10.1140/epjd/e2011-20072-9 |
| Online Access: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1140/epjd/e2011-20072-9 Verlag, lizenzpflichtig, Volltext: https://link.springer.com/article/10.1140/epjd/e2011-20072-9 |
| Author Notes: | J. Deiglmayr, M. Repp, O. Dulieu, R. Wester, and M. Weidemüller |
| Summary: | We investigate the rovibrational population redistribution of polar molecules in theelectronic ground state induced by spontaneous emission and blackbody radiation. As amodel system we use optically trapped LiCs molecules formed by photoassociation in anultracold two-species gas. The population dynamics of vibrational and rotational states ismodeled using an ab initio electric dipole moment function and experimental potentialenergy curves. Comparison with the evolution of the v″ = 3 electronicground state yields good qualitative agreement. The analysis provides important input toassess applications of ultracold LiCs molecules in quantum simulation and ultracoldchemistry. |
|---|---|
| Item Description: | Gesehen am 03.05.2022 |
| Physical Description: | Online Resource |
| ISSN: | 1434-6079 |
| DOI: | 10.1140/epjd/e2011-20072-9 |