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Regio- and diastereoselective transition metal-free hydroalkylation of N-allenyl sulfonamides by push-pull 2-alkynylquinolines

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We describe a novel and efficient synthetic strategy to construct the linear homoallylic quinolone structures through the intermolecular addition of 2-alkynylquinoline to N-allenyl sulfonamides. We developed the regio- and diastereoselective transition metal-free hydroalkylation of 1,2-dienes by a s...

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Bibliographic Details
Main Authors: Dehghanpour Kalan, Reza (Author) , Amiri, Kamran (Author) , Rominger, Frank (Author) , Balalaie, Saeed (Author) , Bijanzadeh, Hamid Reza (Author)
Format: Article (Journal)
Language:English
Published: 07 Oct 2022
In: Organic & biomolecular chemistry
Year: 2022, Volume: 20, Issue: 42, Pages: 8269-8272
ISSN:1477-0539
DOI:10.1039/D2OB01362B
Online Access:Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1039/D2OB01362B
Verlag, lizenzpflichtig, Volltext: https://pubs.rsc.org/en/content/articlelanding/2022/ob/d2ob01362b
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Author Notes:Reza Dehghanpour Kalan, Kamran Amiri, Frank Rominger, Saeed Balalaie and Hamid Reza Bijanzadeh
Description
Summary:We describe a novel and efficient synthetic strategy to construct the linear homoallylic quinolone structures through the intermolecular addition of 2-alkynylquinoline to N-allenyl sulfonamides. We developed the regio- and diastereoselective transition metal-free hydroalkylation of 1,2-dienes by a structure containing a push-pull system. Moreover, the present work was carried out with a high atom economy, mild reaction conditions, and moderate to high yields.
Item Description:Gesehen am 09.12.2022
Physical Description:Online Resource
ISSN:1477-0539
DOI:10.1039/D2OB01362B

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