State-resolved femtosecond phase control in dense-gas laser-atom interaction enabled by attosecond XUV interferometry

We perform an interferometric measurement of an extreme ultraviolet (XUV) pulse passing through a dense gas-phase target. Utilizing the interaction with strong and narrow atomic resonances, we demonstrate the femtosecond phase control of the resonant XUV pulse propagation by means of a time-delayed...

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Bibliographic Details
Main Authors: Hedewig, Lina (Author) , Kleine, Carlo (Author) , He, Yu (Author) , Wieder, Felix (Author) , Ott, Christian (Author) , Pfeifer, Thomas (Author)
Format: Article (Journal)
Language:English
Published: 29 April 2025
In: Optics letters
Year: 2025, Volume: 50, Issue: 9, Pages: 1-4
ISSN:1539-4794
DOI:10.1364/OL.559945
Online Access:Verlag, kostenfrei, Volltext: https://doi.org/10.1364/OL.559945
Verlag, kostenfrei, Volltext: https://opg.optica.org/abstract.cfm?URI=ol-50-9-3006
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Author Notes:Lina Hedewig, Carlo Kleine, Yu He, Felix Wieder, Christian Ott, and Thomas Pfeifer
Description
Summary:We perform an interferometric measurement of an extreme ultraviolet (XUV) pulse passing through a dense gas-phase target. Utilizing the interaction with strong and narrow atomic resonances, we demonstrate the femtosecond phase control of the resonant XUV pulse propagation by means of a time-delayed intense near-infrared (NIR) laser pulse. XUV spectral interferometry provides direct access to the amplitude and phase of the transmitted pulse and thus enables the full reconstruction of the ultrafast dynamics. We benchmark our measurement approach with the singly excited 1 - s - 4 - p - Rydberg state of helium to directly reconstruct the temporal structure of the transmitted XUV pulse beyond the single-atom response. An NIR-intensity-controlled variable phase step between 0 and 2 rad is measured on the XUV pulse after passage through the medium, originating from laser-induced transient Stark shifts.
Item Description:Gesehen am 25.08.2025
Physical Description:Online Resource
ISSN:1539-4794
DOI:10.1364/OL.559945